Redox regulation of SurR by protein disulfide oxidoreductase in ThermococcusonnurineusNA1

Jae KyuLim1,2·Hae-Chang Jung1,2·Sung GyunKang1,2·Hyun Sook Lee1,2

Sung Gyun Kang · Hyun Sook Lee

e-mail:,

1 Marine Biotechnology Research Division, Korea Institute of Ocean Science and Technology, Ansan15627, Republic of Korea

2 Department of Marine Biotechnology, Korea University of Science and Technology, Daejeon 34113, Republic of Korea

Running title: Reduction of SurR by protein disulfide oxidoreductase

Supplementary material accompanies this paper.

Table S1Sequences of the oligonucleotide primers used for PCR amplification.

Primer / Location / Oligonucleotide sequence
Gene cloning
prnTON0470F / TON_0470 forward / 5'- TGCCGCGCGGCAGCCATATGAGGAGGACTGCTTTACTGTTG-3'
prnTON0470R / TON_0470 reverse / 5'- TGGTGGTGGTGGTGCTCGAGGCGCCTTCTCCTCAGGAG-3'
prnTON0472F / TON_0472 forward / 5'- TGCCGCGCGGCAGCCATATGGACGAGCTGGAGATGATC-3'
prnTON0472R / TON_0472 reverse / 5'- TGGTGGTGGTGGTGCTCGAGCTGTAGGCCTAGCAGCATCC-3'
prnTON0834F / TON_0834 forward / 5'- TGCCGCGCGGCAGCCATATGATCAGGGAGTTTGATGGAG-3'
prnTON0834R / TON_0834 reverse / 5'- TGGTGGTGGTGGTGCTCGAGGGAGTCAGAACCCAGGAGC-3'
prnTON0318F / TON_0318 forward / 5'- TGCCGCGCGGCAGCCATATGACTGAACCGGACATCTTTTAC-3'
prnTON0318R / TON_0318 reverse / 5'- TGGTGGTGGTGGTGCTCGAGATCTTCTCCGGCATCTTCGAC-3'
EMSA DNA probe
prnPmbhF / mbh promoter forward / 5'-CATCCAATTAGGTTTGGGAAATGGT-3'
prnPmbhR / mbh promoter reverse / 5'-AAGGCGGCAATAAATGCCATCTTTC-3'

1

Table S2 Conservation of genes encoding Trx- or Grx-like proteins in the genomes of the order Thermococcales

Genome / Homologues of T. onnurineus NA1 protein (% identity)
TON_0319 / TON_0470 / TON_0472 / TON_0834
Thermococcalesarchaeon44_46 / XD43_0781 (77.7) / XD43_1009 (39.5) / XD43_1823 (80.9) / - b
ThermococcusbarophilusMP / TERMP_00657 (81.7) / TERMP_RS04160 (38.8) / TERMP_00838 (76.7) / TERMP_01376 (51.5)
Thermococcuscelericrescens / APY94_12140 (91.6) / APY94_05295 (60.6) / APY94_05305 (85.2) / APY94_01785 (49.5)
Thermococcuscleftensis / CL1_0385 (93.8) / CL1_0213 (63.1) / CL1_0211 (87.9) / -
Thermococcuseurythermalis / TEU_06555 (90.3) / TEU_08320 (48.2) / - / -
ThermococcusgammatoleransEJ3 / TGAM_1302 (89.8) / TGAM_1636 (42.8) / - / -
ThermococcusguaymasensisDSM 11113 / X802_10250 (84.1) / X802_01105 (46.0) / - / -
ThermococcuskodakarensisKOD1 / TK1085 (88.5) / TK1208 (53.3) / - / TK0838 (50.5)
ThermococcuslitoralisDSM 5473 / OCC_08455 (78.1) / OCC_10925 (40.8) / OCC_13031 (79.1) / OCC_05726 (53.5)
Thermococcus nautili / BD01_0185 (87.2) / BD01_0376 (47.7) / BD01_0378 (88.7) / -
Thermococcusparalvinellae / TES1_0610 (83.0) / TES1_0848 (40.4) / TES1_0851 (77.6) / TES1_1390 (87.4)
Thermococcuspeptonophilus / A0127_09800 (88.5) / A0127_08885 (48.5) / A0127_00965 (83.5) / A0127_10085 (53.5)
Thermococcussibiricus / TSIB_0991 (72.8) / TSIB_RS09715 (37.4) / TSIB_1746 (77.4) / TSIB_1703 (50.5)
Thermococcussp. 4557 / GQS_03675 (91.2) / GQS_02835 (51.9) / - / -
Thermococcusthioreducens / AMR53_03845 (91.6) / AMR53_01730 (60.3) / AMR53_01740 (85.2) / AMR53_05300 (50.0)
Thermococcuszilligii / WP_010478330a (80.4) / WP_010478037a(49.2) / WP_010479774a(83.5) / -
PyrococcusabyssiGE5 / PAB2245 (83.5) / PAB1651 (30.3) / - / -
Pyrococcus furiosus DSM 3638 / PF0094 (80.5) / PF0724 (43.2) / PF1457 (80.7) / PF0741 (47.0)
PyrococcushorikoshiiOT3 / PH0178 (82.1) / PH1130 (34.0) / - / -
Pyrococcus sp. NA2 / PNA2_0698 (83.6) / PNA2_1761 (36.0) / - / -
Pyrococcussp. ST04 / Py04_0249 (84.5) / Py04_1135 (36.1) / - / Py04_0921 (48.5)
PyrococcusyayanosiiCH1 / PYCH_16300 (88.0) / PYCH_08480 (43.6) / PYCH_08820 (80.9) / PYCH_09150 (50.5)
Palaeococcusferrophilus / WP_048148193a(80.4) / WP_048150379a(50.2) / WP_048147785a(78.3) / WP_048147736a(50.5)
PalaeococcuspacificusDY20341 / PAP_07225 (80.4) / PAP_09015 (55.5) / PAP_08980 (76.1) / PAP_08695 (78.6)

a NCBI ( reference sequence accessionnumber was used instead of Locus tag.

b- means no detection

1

Fig.S1 Phylogenetic tree of Trx- or Grx-like proteins. The tree was constructed using the Mega 7 program with the neighbor-joining method with 500 bootstrap replicates. Species name along with the locus tag or NCBI reference sequence accession number are indicated at the termination of each branch.

A. TON_0319 homologue

PAP_07225 --MGLISDGDKKVIREEFFSKLTNPVKIIVFIGKDHCQYCEQLKQLVQEVSELSDLVSYE58

TERMP_00657 --MGLISDGDKKVIREEFFSKLTNPVKLIVFIGKDHCQYCEQLKQLVQEISELSDLVSFE58

TES1_0610 --MGLISDGDKKVIKEEFFSKLTNPVKLIVFVGKEHCQYCEQLKQLVQEISELSDLVSYE58

TSIB_0991 --MALISDGDKKIIKEEFFSKLVNPVKLLVFIGKDHCQYCDQLKQLVEEISELSDLVTYE58

XD43_0781 --MALISDGDKKIIKEEFFSKLVNPVKLIVFTGKEHCQYCDQLKQLVEEISELSDLISYE58

OCC_08455 MEMALISDGDKKIIKEEFFSKLVNPVKIIVFTGKEHCQYCDQLKQLVEEISELSDLISYE60

WP_048148193 --MGLISDGDKKVIKEEFFSKLEEPVKLIAFIGKEHCQYCDQLKQILAEISELSDKVTYE58

WP_010478330 --MGLISDADKRVIKEEFFSRLTNPVKLMVFTGREHCQYCTQLKQLVQELSELTDKLTYE58

PF0094 --MGLISDADKKVIKEEFFSKMVNPVKLIVFVRKDHCQYCDQLKQLVQELSELTDKLSYE58

Py04_0249 --MGLISDADKKIIKEEFFSKMTNPVKLIVFIGKEHCQYCDQLKQLVQELSELSDKLTYE58

PNA2_0698 --MGLISEEDKRIIKEEFFSKMVNPVKLIVFIGKEHCQYCDQLKQLVQELSELTDKLSYE58

PAB2245 --MGLISEEDKRIIKEEFFSKMVNPVKLIVFIGKEHCQYCDQLKQLVQELSELTDKLSYE58

PH0178 --MGLISEEDKRIIKEEFFSKMVNPVKLIVFIGKEHCQYCDQLKQLVQELSELTDKLSYE58

PYCH_16300 --MGLISEEDKKVIREEFFSKMTNPVKLIVFVGKEHCQYCDQLKQLVQELSELTDKLTYE58

X802_10250 --MGLISDADKKVIKEEFFSKLTEPVKLMVFTGKEHCQYCDQLKQLVQELAELSDKLTYE58

BD01_0185 --MGLISDADKKVIKEEFFSKLTEPVKLMVFIGKDHCQYCDQLKQLVQELAELSDKLSYE58

TK1085 --MGLISDADKKVIKEEFFSKMTNPVKLIVFVGKEHCQYCDQLKQLVQELSELTDKLSYE58

A0127_09800 --MGLISDADKKVIKEEFFSKMTNPVKLIVFVGKEHCQYCDQLKQLVQELSELSDKLSYE58

AMR53_03845 --MGLISDADKKVIREEFFSKMTNPVKIIGFIGKEHCQYCDQLKQLVQELADLSDKLTYE58

TEU_06555 --MGLISDADKKVIKEEFFSKLTNPVKIIGFIGKDHCQYCDQLKQVVQELSELTDKLTYE58

APY94_12140 --MGLISDADKKVIREEFFSKMTNPVKIIGFIGKEHCQYCDQLKGLVQELSELSDKLTYE58

GQS_03675 --MGLISDADKKVIKEEFFSKMTNPVKIIGFTGKEHCQYCDQLKGLVQELSELTDKLTYE58

TGAM_1302 --MGLISDADKKIIKEEFFSKMTNPVKIIGFTGKEHCQYCDQLKQLVQELSELTDKLTYE58

CL1_0385 --MGLISDNDKKVIKEEFFSKLTNPVKIIGFIGKDHCQYCDQLKQLVQELSELTDKLTYE58

TON_0319 --MGLISDGDKKVIREEFFSKMTNPVKIIGFIGKDHCQYCDQLKQLVQELSELSDKLSYE58

*.***: **::*:*****:: :***:: * ::***** *** :: *:::*:* :::*

PAP_07225 IHDFDNE--KELAEKYRIDKAPSLVITQDGKDLGVRYFGLPAGHEFGAFLEDIVDVSNGT116

TERMP_00657 VHDFDTE--KELAQRYRVDRAPVTVITQDGKDFGVRYFGLPAGHEFGAFLEDIVDVSNGT116

TES1_0610 IHDFDTE--KELAEKYRIDRAPATIITQDGKDLGVRYFGLPAGHEFGAFLEDIVDVSNGT116

TSIB_0991 LHDFDSE--KELAEKYRIDIAPAVVMTQNGKDLGVRYFGLPAGHEFGSFLEDIVDVSKGE116

XD43_0781 IHDFDSE--KELAEKYRVDRAPVTIITQDGKDLGVRYFGLPAGHEFGSFLEDIVDVSRGE116

OCC_08455 VHDFDSE--KELAEKYRIDKAPVTIITQDGKDFGVRYFGLPAGHEFGSFLEDIVDVSKGE118

WP_048148193 VHDFDAE--KELAEKYRVDRAPATVITRNGEDFGVRFFGLPAGHEFGAFLEDIVDVSTGN116

WP_010478330 FHNFDTPEGKEIARKYRIDRAPAVTITQDGKDMGVRYFGLPAGHEFGSFLEDIVDVSNGT118

PF0094 IVDFDTPEGKELAKRYRIDRAPATTITQDGKDFGVRYFGLPAGHEFAAFLEDIVDVSREE118

Py04_0249 IVDFDTPEGQELARKYRIDRAPATTITQDGKDFGVRYFGLPAGHEFAAFLEDIVDVSNAQ118

PNA2_0698 IIDFDTPEGKELAKKYRIDRAPATTITQDGKDFGVRYFGIPAGHEFAAFLEDIVDVSRAD118

PAB2245 IVDFDTPEGKELAEKYRIDRAPATTITQDGKDFGVRYF--PAGHEFAAFLEDIVDVSRAE116

PH0178 IVDFDTPEGKELAEKYRIDRAPATTITQDGKDFGVRYF--PAGHEFAAFLEDIVDVSKGD116

PYCH_16300 VYDFDTEEGRKIAEQYKVDRAPAVTITQDGRDMGVRYFGLPAGHEFAAFLEDIVDVSNAQ118

X802_10250 FIDFDTEEGKRKAEEYRIDHAPAVSITRNGQDVGVRFFGLPAGHEFGAFLEDIVDVSNMT118

BD01_0185 VIDFDTEEGKKKAEEYRIDRAPAVSITRNGQDVGVRFFGLPAGHEFGAFLEDIVDVSNMT118

TK1085 VVDFDTEEGKKLAEQYRIDRAPATTITQDGKDMGVRYFGLPAGHEFGAFLEDIVDVSNGT118

A0127_09800 VVDFDTEEGKKLAEQYRIDRAPATTITQDGRDMGVRFFGLPAGHEFGAFLEDIVDVSNGT118

AMR53_03845 FHDFDSEEGRKLAEQYKIDRAPAVTITQDGRDMGVRFFGLPAGHEFGAFLEDIVDVSNAT118

TEU_06555 FHDFDSEEGRKVAEQYRIDRAPAITITQDGKDMGVRYFGLPAGHEFGALLEDIVDVSNAT118

APY94_12140 FHDFDSEEGRKLAEQYRIDRAPAITLTQDGKDMGVRFFGLPAGHEFGAFLESIVDVSNAT118

GQS_03675 FHDFDTEEGRKIAEQYRIDRAPAITLTQDGKDMGVRFFGLPAGHEFGAFLESIVDVSNAT118

TGAM_1302 FYDFDTEEGRKVAEQYRIDRAPAVTITHDGKDVGVRFFGLPAGHEFSAFLEDIVDVSNMT118

CL1_0385 FHDFDSEEGRKLAEQYRIDRAPAVTITQDGKDMGVRFFGLPAGHEFGAFLEDIVDVSNAS118

TON_0319 FYDFDSEDGRKLAEQYGIDRAPAITITQDGKDMGVRFFGLPAGHEFGAFLEDIVDVSNAQ118

. :** :. *..* :* ** :*::*.*.***:* ******.::**.*****

PAP_07225 TDLMPETKEALKNIDKDVQIYAFVTPTCPYCPMAVRMAHKFAIENALAGKGKILGDMIEA176

TERMP_00657 TDLMKETKETLKEIDRDVRILVFVTPTCPYCPMAVRMAHKFALENALAGKNKILGDMVEA176

TES1_0610 TDLMPDTKDTLKSIDKDVRILVFVTPTCPYCPMAVRMAHKFAIENALAGKGKILGDMVEA176

TSIB_0991 TDLSEETKEALKEINKDVQIYVFVTPTCPYCPMAVRMAHKFAIEHALAGNDRILGDMIEA176

XD43_0781 TDLSEETKEAVRNIDRDVEIYVFVTPTCPYCPMAVRMAHKFAIENALAGKGKILGDMIEA176

OCC_08455 TDLMEDTKEAVRNIDQDVEIYVFVTPTCPYCPMAVRMAHKFAIENSLAGKGKILGDMIEA178

WP_048148193 TDLAPDTKEAIANVERDVRILVFVTPTCPYCPMAVRMAHKFALENTKAGKGKILGDMVEA176

WP_010478330 TDLMPESKKALH--ERDVRILVFVTPTCPYCPLAVRMAHKFAIENAIAGKGRILGDMVEA176

PF0094 TNLMDETKQAIRNIDQDVRILVFVTPTCPYCPLAVRMAHKFAIENTKAGKGKILGDMVEA178

Py04_0249 TDLMDESKEALRNIDQDVRILVFVTPTCPYCPLAVRMAHKFAIENTKAGKGKILGDMVEA178

PNA2_0698 TDLMPDSKEEVAKIDKDVRILVFVTPTCPYCPLAVRMAHKFAIENTKAGKGKILGDMVEA178

PAB2245 TDLMAESKEEVAKIDKNVRILVFVTPTCPYCPLAVRMAHKFAIENTKAGKGKILGDMVEA176

PH0178 TDLMQDSKEEVSKIDKDVRILIFVTPTCPYCPLAVRMAHKFAIENTKAGKGKILGDMVEA176

PYCH_16300 TDLMPDTKETIR--DRDVRILVFVTPTCPYCPMAVRMAHKFAIENTNAGKGKIKGDMVEA176

X802_10250 TDLMPDTKEAIANVDRDVRILVFVTPTCPYCPLAVRMAHKFAVENTKAGKGRILGDMVEA178

BD01_0185 TDLMPESKEALAKIDRDVRILVFVTPTCPYCPLAVRMAHKFAIENTNAGKGKILGDMVEA178

TK1085 TDLAPDTKEAIHGVDKDVRILVFVTPTCPYCPLAVRMAHKFAIENTLAGKGKILGDMVEA178

A0127_09800 TDLAPDTKEAIHGVDKDVRILVFVTPTCPYCPLAVRMAHKFAIENTLAGKGKILGDMVEA178

AMR53_03845 TDLMPDSKEELAEIDRDVRILVFVTPTCPYCPLAVRMAHKFAIENAKAGKGRILGDMVEA178

TEU_06555 TDLMQETKEAIANVERDVRILVFVTPTCPYCPLAVRMAHKFAIENTNAGKGKILGDMVEA178

APY94_12140 TDLMPESKQDLANVDRDVRILVFVTPTCPYCPLAVRMAHKFAIENTNAGKGRILGDMVEA178

GQS_03675 TDLMPESKEELAKVDRDVRILVFVTPTCPYCPLAVRMAHKFAIENTNAGKGKILGDMVEA178

TGAM_1302 TDLMPESKEALAKIDRDVRILVFVTPTCPYCPLAVRMAHKFAIENTNAGKGRILGDMVEA178

CL1_0385 TDLMPESKEELAKIDRDVRILVFVTPTCPYCPLAVRMAHKFAIENTNAGKGKILGDMVEA178

TON_0319 TDLMPDTKEELAKVDRDVRILVFVTPTCPYCPLAVRMAHKFAIENTNAGKGKIRGDMVEA178

*:* ::*. : :::*.* **********:*********:*:: **:.:* ***:**

PAP_07225 IEYPELADKYSVMAVPKVVIRVNGEDKVSFEGAYPEKMFLEKLMEALE224

TERMP_00657 IEYPEWADQYRVMAVPKIVIQVDGVDKVEFEGAYPEKMFLEKLLEALE224

TES1_0610 IEYPEWADQYRVMAVPKIVIQVDGVDKVEFEGAYPEKMFLEKLLEALE224

TSIB_0991 IEFPELAEQYGVMAVPKVVIKVNGEDKISFEGAYPEKMFLEKLLEALE224

XD43_0781 IEFPEWADQYSVMAVPKVVIRVDGEDKVSFEGAYPEKMFLEKLLQALE224

OCC_08455 IEFPEWADQYSVMAVPKVVIRVNGEDKVSFEGAYPEKMFLEKLLQALE226

WP_048148193 IEYPEWADEYKVMAVPKVVIMVDGEDKVQFEGAYPEKMFLEKLLAALE224

WP_010478330 IEYPEWADEYSVMAVPKIVIQVDGEDRVEFEGAYPEKMFLEKLLAALE224

PF0094 IEYPEWADQYNVMAVPKIVIQVNGEDRVEFEGAYPEKMFLEKLLSALS226

Py04_0249 IEYPEWADQYNVMAVPKIVIQVNGEDKVQFEGAYPEKMFLEKLLAALS226

PNA2_0698 IEYPEWADQYNVMAVPKIVIQVNGEDKVQFEGAYPEKMFLEKLLAALS226

PAB2245 IEYPEWADQYNVMAVPKIVIQVDGEDKVQFEGAYPEKMFLEKLLAALS224

PH0178 IEYPEWADQYNVMAVPKIVIQVNGEDKVQFEGAYPEKMFLEKLLSALS224

PYCH_16300 MEYPEWADQYNVMAVPKIVIQVDGEDKVQFEGAYPEKMFVEKLLAALG224

X802_10250 IEYPEWADQYSVMAVPKIVIQVDGEDKVQFEGAYPEKMFMEKLLTALE226

BD01_0185 IEYPEWADQYSVMAVPKIVIQVDGEDKVQFEGAYPEKMFMEKLLAALE226

TK1085 IEYPEWADQYSVMAVPKIVIQVDGEDKVQFEGAYPEKMFLEKLLAALE226

A0127_09800 IEYPEWADQYSVMAVPKIVIQVDGEDKIQFEGAYPEKMFLEKLLAALE226

AMR53_03845 IEYPEWADQYSVMAVPKIVIQVDGEDKVQFEGAYPEKMFMEKLLAALS226

TEU_06555 IEYPEWADQYSVMAVPKVVIQVDGEDKVQFEGAYPEKMFLEKLLAALE226

APY94_12140 IEYPEWADKYSVMAVPKIVIIVDGEDKVQFEGAYPEKMFMEKLLAALE226

GQS_03675 IEYPEWADKYSVMAVPKIVIIVDGEDKVQFEGAYPEKMFMEKLLAALE226

TGAM_1302 IEYPEWADQYSVMAVPKIVIQVDGEDKVQFEGAYPEKMFMEKLLAALE226

CL1_0385 IEYPEWADQYSVMAVPKIVIQVDGEDKVQFEGAYPEKMFMEKLLAALE226

TON_0319 IEYPEWADQYSVMAVPKIVIQVDGEDKVQFEGAYPEKMFMEKLLAALE226

:*:** *::* ******:** *:* *::.**********:***: **

B. TON_0470 homologue

TSIB_RS09715 ---MKRIVVSLLIM---MMVFISMCISNNTSTSST------29

XD43_1009 ---MKKVLTGLLLV---LVVLTSMCISDNPSSSSS------29

OCC_10925 ---MKKVLTGLLLV---LVVLTSMCISDNPSSSSS------29

TES1_0848 ---MRRILNGILIV-LVLSTVMSMCISNNSSTSTQIASTSNSQATVSTTQVLTTTSTIQS56

TERMP_RS04160 ---MKRIVAGVVFAVVILGVFASLCISNNNTMTSPSAM------Q-36

PYCH_08480 ----MKELSILL--IIILAVAALGCLGETSTPTTSPP------31

Py04_1135 ---MNRVPIILL--VFVLPIVISGCISSPPSTQTISQHAST------36

PH1130 ---MKRDLALLL--ILVLAASFLGCISSQ------24

PAB1651 ----MKKVAFIL--IIVLLAFSLGCLSSTSTPTTTQT--SQ------33

PNA2_1761 ----MRKAFTVI--LLILLTSSLGCLSSN------23

PF0724 ---MKLKAL-FL--LLALGSLIVPRI------20

CL1_0213 ---MRKTGVVLV--LLLIVGVASGCISNSNGPTA---TQT------32

GQS_02835 ---MKKFGIVLL--IILLAGFAAGCISNSGGSNTSSTTQT------35

TK1208 ---MKKTGILLM--LLVLVGFASACLSSDSN--TSS---Q------30

A0127_08885 ---MKKTGILLM--LLVLVGFASACLGSDSN--TSS---Q------30

TEU_08320 ---MKKVGVLLL--LLFLIGFSAGCIGSDNTDTTSS---T------32

BD01_0376 ---MKKAGVLLL--LLVLLGFSAGCIGSNGTTGTSS---T------32

WP_010478037 ---MKVPRALLA--LTLSLAFLALPVASA------24

TGAM_1636 MAGMKRVV-GLA--LLLLLSSVLFPV-SA------25

X802_01105 ---MKRFVMSAT--LLLLVSSMLLPIASA------24

TON_0470 ---MRRTALLLL--FLLTVSLLSYAV------21

APY94_05295 ---MRKLVLIII--GMLLISTVSYAV------21

AMR53_01730 ---MKKLVLFFI--WLLVFSTVSYAL------21

WP_048150379 ---MRKLYGLVI--LLIVLSTLSHAL------21

PAP_09015 ---MRKAALFIV--FLFLASAVSLVL------21

:

TSIB_RS09715 --PTTNPT---ETTNPLTLDKSKFHFYEYGLATCPHCRKMKEELPKAFGKEALTYYELQG84

XD43_1009 --PS------TATETFTLDKAKFHFYMYGLATCPHCKKMKEEIPKFFGKDALTYYELQG80

OCC_10925 --PS------TATETFTLDKAKFHFYMYGLATCPHCKKMKEDIPEFFGEEALTYYELQG80

TES1_0848 SGPSSTET---TSTHEQNIDITKLHFYMFGVSTCPHCGKMKQLLPEIFGKDKFTYYELQG113

TERMP_RS04160 --SSSVNT---QTQSQNQIDVSKLHFYMFGLATCPHCKKMKQLLPEAFGKNSLTYYELQG91

PYCH_08480 ------KLQLDKSKFHFYLYGMATCPHCQNMKRELPKFFGEDSLTYYELIN76

Py04_1135 -TPTSHQSTTITEDWLEGLDKSKFHFYIYGLDTCPHCQRMKELLPEYFGEGSLTFYEVRK95

PH1130 -----TQTQTSQEKWLEGLKKSEFHFYIFGLNTCPHCQRMKKLLPEYFGNSSLTFYEIRE79

PAB1651 -PSPTTPSKTQAQDWLEGLDKSKFHFYVFGVNTCPHCRRMKELLPEYFGNKSLTFYEVRE92

PNA2_1761 -----TPTQTKTESWLEGLEKEKFHFYMFGVNTCPHCQKMKRLLPEYYGNGSLTFYELRE78

PF0724 ------EAEEFESSKVHFYMYGAYWCPHCRNVKESIKEHFGEETLTYYEIEG66

CL1_0213 ---TTSSIPDYVVVNGTKIYLDEIHFYMYGMKTCPHCQNMKKLIPETYGEDSLTYYELVD89

GQS_02835 ---TSSGGSDYVVVNGTKIYLDDIHFYMYGMKTCPHCHKMREEISETYGEDSLTYYELVD92

TK1208 ---TSTESPKYVDVNGTRIYLDQIHFYMYGMKTCPHCRHMKEWIPEEFGADSLTYYELVN87

A0127_08885 ---TSTESPKYVDVNGTKIYLDQIHFYMYGAKTCPHCRNMKTQIPSVYGEDALTYYELID87

TEU_08320 ---STAAQQDYVDVNGTKIYLDKVHFYMYGAKTCPHCRNMKEKIPAKYGEEAFTYYELVN89

BD01_0376 ---STTSKPAYVDVNGTRIYLNEIHFYMYGMKTCPHCRHMHEWIPQEYGEKALTYYELVG89

WP_010478037 ------SDWKFDKSKVHFYMYGLSTCPHCRNMKQLIPEVYGSDKLTYYELNG70

TGAM_1636 ------SDWKFDPSLVHFYLYGAKTCPHCRHMKEVIPETYGADKFTYYELVG71

X802_01105 ------SEWKFDPSLVHFYMYGAKTCPHCRHMKELIPATYGSDKFTYYELTG70

TON_0470 ------AETQIDSNKVHFYMYGMSTCPHCQNMKKLIPEIYGPESLTYYELVN67

APY94_05295 ------AEGQVNPDKLDFYMYGAKTCPHCRKMKEEIPRVYGNDSFTYYELVD67

AMR53_01730 ------VETQIDPGKLHFYMYGLETCPHCQKMKEEIPKFYGENSLTYYELIN67

WP_048150379 ------AQGEIDPKKVHFYMYGAATCPHCKKMKEEIPKAFGADSLTYYELVN67

PAP_09015 ------ADTQIDKSKVHFYMYGTKTCPHCKKMKEEIPKQFGEQSLTYYELID67

. ..** :* **** .:: : :* :*:**:

TSIB_RS09715 NDHNNQMFNQLYEILGVTTVPVIGIFYDGKLYAIVNGEFPTDY--ADDFVEEAMKAKGVL142

XD43_1009 NEHNGKMFEQLYEILGVTGVPVIGVFYEGKLYAIVNGEFPVDY--ADDLVEEAKKAEGVL138

OCC_10925 NEHNGKMFEQLYEILGVTGVPVIGVFYEGKLYAIVNGEFPVDY--ADDLVEEAKKAEGVL138

TES1_0848 NEHNTQLFSELYNILGVTGVPVIGIFYDNHLVAVIEGEIPDPAKNVPWLVNTALKENGVL173

TERMP_RS04160 NDHNSNLFSELYSMLGVTGVPVIGIFYDNRLVAIVEGEIPEPSKNVPIIVETAIKEKGVL151

PYCH_08480 NEHNTKIFMEFSKELGVRGVPLIGVFYDGKLYAIIEGEIDP--SKIPEIVKEAMDREGII134

Py04_1135 SEKNFEIYQNFSKMIGVTGVPLIGVFYSGKLYAIIEGEIDP--KVIPKIVKTAMEHNSVI153

PH1130 DKKAYNTYMKFVKTLGITGVPLIGIFYKDNLYAVVEGEIDP--KVIPQLVKEAMKNNGVI137

PAB1651 NKTAYEFYLKFMETLGVTGVPLIGIFYENKLYAVVEGEIDP--RDIPKLVKAAMKENGVA150

PNA2_1761 NKKAYEFYLNFATTLKITGVPLIGIFYDNKLYAIVEGEIDP--KVIPRIVKEAMKDNGVI136

PF0724 VEHNKNKFEELYLLTGISGIPATAIFYEGEIYAVIEGEFDV--SKTWQIITEAKNQGGVI124

CL1_0213 NEENTKLFQQIYQLTGIQGVPAIAITYNGTLYAIIEGEFNV--TATPRIIQAAMSDNGVI147

GQS_02835 NEENSKLFQRIYQITGIQGVPAIAITYNGTLYAVLEGEFNV--TAVPKIIYTGMKNNGAI150

TK1208 DETNSELFGQLAQLTGITGVPAIAITYNGTIQAIFEGEFNV--SATPEIVATAMNANGVI145

A0127_08885 NETNMELFRQLNQLTGITGVPAIAIVYNDSLQAIFEGEFKV--NATPEIIATAMKENGVI145

TEU_08320 NQTNMELFNQLAQLTGITGVPAIAIAYNGTLYAVIEGEFDV--EKAPEIIATAMENNGVF147

BD01_0376 NQTNMMLFNELAQLTGITGVPAIAITYNGTLYAVIEGEFNV--TATPEIIATAIKNDGVL147

WP_010478037 NQYNIRAFNNISSLTGITGVPAIGIVYDGQLVAVIEGEFNV--SATPEIVKAAIDRNGTI128

TGAM_1636 NSHNDEVLNNISRLIGVTGVPVIGITYNGTLVAVIEGEYKV--SATPEIVETALKNNGTL129

X802_01105 NNHNINVFGNISRLTGITGVPAIGIVYNGTLVAVIEGEYNV--SATPEIIKAAIENHGML128

TON_0470 NEENQKLFGEQYKYTGIMGVPAVAITYNGTLYAIIEGEFNV--SATPEIIEAAMENNGLI125

APY94_05295 NTENQALFGEQYRYTGISGVPAIGIAYEGELRAIVEGEFNV--SAAPKIVEAAIENDGLI125

AMR53_01730 NDENNKLFSAQYKYTGIAGVPAIGIAYDGKLVAIVEGEYNV--SATPKIVQAALDNGGLI125

WP_048150379 NDENSALFGEIYRLTGISGVPAIGIAYDGKLYAIIEGEFNV--SATPEIIKEAQERNGMF125

PAP_09015 NEENGALFSEVYQLTGISGVPAIGIAYDNKLYAIIEGEFNV--SATTEIIKTAQENNGLI125

: :* .: *.. : *:.:** :: . . .

TSIB_RS09715 F-ITDKVYLIPGNNTEII---NKLESIFTNGEPSEV------174

XD43_1009 F-ITDKTYLIPENQTEII---NKLEYIFTNGEPSEV------170

OCC_10925 F-ITDKTYLIPENQTEII---NKLEYIFTNGEPSEV------170

TES1_0848 F-IADKTYLFPSNQTETI---KKLENIFMNGEPSEG------205

TERMP_RS04160 F-ITDKTYLIPLNQTETI---KKLENIFMNGEPSEG------183

PYCH_08480 V-LSSRAYLIPFNETDIV---QKLTELFLSGQASQ------165

Py04_1135 LILSSGQYILPLNNTKAESAVTNMTKWFLMGQPEP------188

PH1130 LIISQGQFLVPKNESKGLELIGNMTTWFKLNGH------170

PAB1651 LIISRGQFLIPRNETKGIEAISNLTSWFKLGEH------183

PNA2_1761 LIISSGQFIIPGNETKI---IGNLTSWFKLGEQ------166

PF0724 LVTSGKAYILKWDSQE----VQKLKEIFLSGKVNET------156

CL1_0213 LFVGGQAYILPRDKEDSAKVIDELYVLFVEHKMPDSS------184

GQS_02835 LAVGGKVYLLPRDKEDSAKVIDELYTLFVEHKMPPQESN------STSD------193

TK1208 LFIGGEWYLLARDNPRSETLIDALQTIFVEHESVDVQSVLTKLKSNSTG------194

A0127_08885 MVVQGQIYLLPRNDPRYSALIDALRTIFVEHRGVDVQSVLEKLKSNSTG------194

TEU_08320 LI-VGKVYLLPRDEPKWKLVIDALHTLFVEHEPVDVQEILDQLKANSTSAG------197

BD01_0376 LL-TGKTYLLSYKDPKAKLVINALYTIFVKHQSVDVQKIFNELKANSTSTG------197

WP_010478037 LLVGGGAYLIPHNTTGGMNLTNALYELFVRPTAT------TT164

TGAM_1636 LLLASGNYILPHNNTKAREIVEKLQYLFTKAGEPSETSTTPKK--THTTASETPADGTHT187

X802_01105 LFVGGRAYILPRNETEAMETIEKLQYLFTRAGEPSKTSTTTKK--THTTTSKATANETHI186

TON_0470 LFVAGQAYIIKNE-----TIIQKLQTIYVEHRLPEADTTETSEITTS-----TPSEDETT175

APY94_05295 LVMGGKAYIIKNE-----TIIQKLQVIYVEHRNPDETVTTTT------TP-TNN-T168

AMR53_01730 LFTGGQAYIIKNE-----TIIQELQAIYVEHRMPGEGQTTTT------TA-SETTS169

WP_048150379 LVTGGKVYLIPRNETEGAQTIAKLETLFIEHRSATGTTGTSPTTTSNTETTETTSTALPT185

PAP_09015 LFVGGKAYILKNE-----THIEMLEKLFIEHKSALNETQTSST------163

. ::. . : :

TSIB_RS09715 ------174

XD43_1009 ------170

OCC_10925 ------170

TES1_0848 ------205

TERMP_RS04160 ------183

PYCH_08480 ------165

Py04_1135 ------188

PH1130 ------170

PAB1651 ------183

PNA2_1761 ------166

PF0724 QKKAEEKSICGPASVLLLSMGAIYLRKRNYSTEVSSNV194

CL1_0213 ------184

GQS_02835 ------193

TK1208 ------194

A0127_08885 ------194

TEU_08320 ----NSTG------201

BD01_0376 ----NSTG------201

WP_010478037 TTSKGGGGICGPATVIGLSAIPILLRRRR------193

TGAM_1636 TTNGNDKRICGPALIIAIAMVPLFPRRRR------216

X802_01105 TTNGNDKRICGPALIIAIAMVPLFLGRNR------215

TON_0470 STSENNDKVCGPGIMAVLVIVPIVLLRRRR------205

APY94_05295 TTSSSDNGICGPGIVVAFAVIPLVLLKRRR------198

AMR53_01730 TTTNPGSEICGPGIAVVLAVLPLVLWKKRR------199

WP_048150379 TTGTNENKTCGPAFIGLLALLPLLMRRANH------215

PAP_09015 -QSPSKEGICGPGLIFAFALVPLLFKRRR------191

C. TON_0472 homologue

PAP_08980 ------MDELEMIRRKKMLELMKRMNGIEK--PKPKVIIEVLTSPTCPYCPIALQMAQ50

TERMP_00838 ------MDELEMIRRKKMLELMKRMGMVEVKPKGPRVVIEVITSPTCPYCPIALQMAK52

TES1_0851 ------MDELEMIRRKKMLELMKKMGMVEVKPKKPRVVIEVITSPTCPYCPIAVQMAQ52

WP_048147785 ------MDELEMIRHKKMLELMRRAGMIEEKPREPKVVIEVITSPGCPYCPIAWAMAQ52

A0127_00965 ------MDELEMIRRKKMLELMKRAGMIEAKPKGPKVIIEVITAPTCPYCPIALQMAK52

PYCH_08820 ------MDELEMIRRKKMLELMKRMGIIEEKPKRPKVTIEVITSPTCPYCPIALAMAQ52

XD43_1823 ------MIRRKKMLELMKKAGMIEEKPRGPKVVIEVITSPGCPYCPIAWAMAQ47

OCC_13031 ------MDELEMIRRKKMLELMKKAGIIEVKPKKPKVIIEVITSPTCPYCPIAWAMAQ52

TSIB_1746 MKFSWGEKMDELEMIRRKKMLELMKKAGIIEVKQEKPKVIIEVITSPGCPYCPIAWAMAQ60

PF1457 ------MIRRKKMLELMKRMGIIEERKPKKKVIIEVITAPGCPYCPIAVQMAR47

WP_010479774 ------MDELEMIRRRKMLELMKRAGMIEGN-KEPKVVIEVITSPGCPYCPIAWAMAQ51

TON_0472 ------MDELEMIRRKKMLELMKRTGMIEVKSKGPKVVIEVITAPGCPYCPIAVQMAR52

BD01_0378 ------MDELEMIRRKKMLELMKRAGMIEVKPKR-KVVIEVITAPGCPYCPIAVQMAK51

AMR53_01740 ------MDELEMIRRKKMLELMKRAGMIDVKPKR-KVVIEVITSPGCPYCPIAWAMAQ51

APY94_05305 ------MDELEMIRRKKMLELMKKAGMIEVTPKK-KVVIEVITSPGCPYCPIAWAMAQ51

CL1_0211 ------MDELEMIRRKKMLELMKRAGMIEVKPKGPKVVIEVITSPGCPYCPIAWAMAQ52

***::******:: . :: :* ***:*:* ******* **:

PAP_08980 EIGRRYQGVEVRELSVATPEGQRKAMEHNIMGVPTILINNKVEFIGVPHPGEFERKVKGY110

TERMP_00838 EIARRHPGVIVKELSVATPEGRKKAMEHNILGTPTILINNKVEFIGVPPFVEFERKVKEK112

TES1_0851 EIARKYQGIVVKELSVATPEGRKKAMEHNILGTPTILINNRVEFIGVPSFVEFERRVKEK112

WP_048147785 ELERRYEGVVAKELSVATPEGRRKAMEHNIMGTPTVLINNRVEFVGVPNFAEFERRVKRH112

A0127_00965 ELERRYEGVVAKEVSVATPEGQRKAMEHNIMGTPTILINNRVEFIGVPNFAEFESRVRAY112

PYCH_08820 EIARKYKGVVARELSIATPEGRRKAMEHNIMGTPTILINNRVEFIGVPNFAEFERKVRQY112

XD43_1823 EIARKYDGVVAKEVSVATPEGQRKAMEHNIMGTPTILINNRVEFIGVPNFAEFERRVRQY107

OCC_13031 EIARKYDGVIAKEVSVATPEGQRKAMEHNIMGTPTILINNRVEFIGVPNFAEFERRVRQY112

TSIB_1746 EIARKYDGIIAKEISVATPEGQRKAREHNIMGTPTILINNRVEFIGVPNFAEFERRVRQY120

PF1457 EIEKKYPGVIVRELSVATPEGRRKAMEHNILGTPTILINNRVEFIGVPRFIDFERRVREL107

WP_010479774 ELERKYDGVIARELSVATPEGRRKAMEHNIMGTPTILINNRVEFIGLPNFAEFERKVREL111

TON_0472 ELERKYNGVVARELSVATPEGQRKAMEHNILGTPTILINNRVEFIGVPNFGEFERKVRML112

BD01_0378 ELEGKYEGVVARELSVATPEGQRKAMEHNILGTPTILIDNRVEFIGVPNFAEFEKRVRER111

AMR53_01740 ELERKYEGVVARELSVATPEGQRKAMEHNIMGTPTILIDNRVEFIGVPNFAEFEKRVREK111

APY94_05305 ELERKYEGVIARELSVATPEGQRKAMEHNIMGTPTILIDNRVEFIGVPNFAEFERRVREK111

CL1_0211 ELERKYEGVIARELSVATPEGQRKAMEHNIMGTPTILIDNRVEFIGVPNFAEFERRVREK112

*: :: *: .:*:*:*****::** ****:*.**:**:*:***:*:* :** :*:

PAP_08980 LGI----113

TERMP_00838 LSSA---116

TES1_0851 LSSV---116

WP_048147785 LSA----115

A0127_00965 LSR----115

PYCH_08820 LSA----115

XD43_1823 LST----110

OCC_13031 LST----115

TSIB_1746 LSA----123

PF1457 LS-----109

WP_010479774 LSDNRKP118

TON_0472 LGLQ---116

BD01_0378 LGLGAPR118

AMR53_01740 LGLK---115

APY94_05305 LGLQ---115

CL1_0211 LGLQ---116

*.

D. TON_0834 homologue

PAP_08695 MIREFDGDFEKVERAKYALLWFSSPGCPPCRMIEPFMHELSEEYENVEFWEVDINKHLAL60

TON_0834 MIREFDGDFGKVERAKYALLWFSSPGCPPCRMIEPFMHELSEEYKEVEFWEVDVEKHLPL60

TES1_1390 MIREFDGDFGKVERAKYALLWFSSPGCPPCRMIEPFMHELSEEYKEVEFWEVDVGKHLWL60

Py04_0921 MIIEYEGKTNFRE--GKVVLWFSIPGCPPCRMVEGFMEELSGEFPEVKIIHVNAGEWDGL58

PF0741 MIIEYDGEIDFTK--GRVVLWFSIPGCPPCRLVERFMTELSEYFEDIQIVHINAGKWKNI58

TSIB_1703 MIHEYDGKIDFNR--GKVVLWFSIQGCPPCRLVESFMEEVSEEFSEIRFIHVGAEKWSNI58

OCC_05726 MIIEYDGKIDFTK--GKVVLWFSIPGCPPCRLVETFMEELSEEFKDIRVIHVHAEKWEDL58

A0127_10085 MIVEYDGKADFTN--GKVVLWFSIPGCPPCRLVESFMEELSDEFREIAIVHVNAEKWSEL58

TK0838 MIVEYDENVDFTK--GKAVLWFSIPGCPPCRLVEAFMKELSEEFGEIAIVHVNAEKWSGL58

WP_048147736 MIVEYDGKVDFEK--GKAVLWFSIPGCPPCRLVENFMKEVSEEFPEIKVIHVNAEEWSDL58

APY94_01785 MIVEYDGKFEFES--RKTVLWFSIPGCPPCRIVESFMEDLSGEFPEIKVVHINAEEWNDL58

AMR53_05300 MIVEYDGKINFMD--GKAVLWFSIPGCPPCRIVDSFMEELSAEFPEITVVHINAEEWNDL58

PYCH_09150 MIVEYDGKINFMD--GKAVLWFSIPGCPPCRIVDSFMEELSAEFPEITVVHINAEEWNDL58

TERMP_01376 MIVEYDGKINFMD--GKAVLWFSIPGCPPCRIVESFMEELSAEFPEITVVHINAEEWNDL58

** *:: . .:**** ******::: ** ::* : :: . .: : :

PAP_08695 IQKFDILNVPTLVYLKEGREVDRQNLIRRKEEVEERIKQLLKG-----103

TON_0834 AEKFDVMNVPTLIYLKEGNEIARQNLVRKKEEVEEKLMMLLGSDS---105

TES1_1390 AEKFDVMNVPTLIYLKEGNEITRQNLVRRREDVENILKDIIES-----103

Py04_0921 VNHFEILNIPTLVYLKDGKEMARQNLIRRKEEVLIQFEEMTRS-----101

PF0741 VDKFNILNVPTLVYLKDGREVGRQNLIRSKEEILKKLKELQE------100

TSIB_1703 VKRFEVLNVPTLVYLKDGKEVARQNLIRSKEEVLAKIEELHEC-----101

OCC_05726 VDKFDILNVPTLVYLKDGKELTRQNLIRTKEEVLLKFEELRES-----101

A0127_10085 VGKF--LNVPTLVYLKDGNEVWRQNLIREKEEVLIKLKELREL-----99

TK0838 VEGFRILNVPTLVYLKDGKEVARQNLIRGKGEVLIKFEEPREL-----101

WP_048147736 VNRFDVLNVPTLVYLKDGKEVARQNLIRNREEVLLRLEELRELQRAGL106

APY94_01785 VNRFDVLNVPTLIYLTDGKEVGRQNLIRKKEEVLIRFEELRRL-----101

AMR53_05300 VNRFDVLNVPTLIYLKDGEEVARQNLIRRK-EVLIRFEELKRL-----100

PYCH_09150 VNRFDVLNVPTLIYLKDGEEVARQNLIRRKEEVLIRFEELKRL-----101

TERMP_01376 VNRFDVLNVPTLIYLKDGEEVARQNLIRGKEEVLIRFEELKRL-----101

* :*:***:**.:*.*: ****:* : :: :

Fig. S2 Multiple sequence alignments of Trx- or Grx-like proteins. Multiple alignments were conducted using the Clustal Omega program on web server ( The locus tag or NCBI reference sequence are identical to those in Table S1 and Fig. S2.

Fig.S3SDS-PAGE analysis of the purified Trx- or Grx-like proteins, Pdo, TON_0834, and TON_0472.3 µg of proteins of Pdo and TON_0834 and 6 µg of proteins of TON_0472 were loaded onto a 15% SDS-PAGE gel. The intact proteinsand fragments of TON_0472 are marked.

Fig.S4Effect of Pdo concentration on the reduction SurR. Reduction of disulfide bonds of 4 µMSurR by 50 nM TrxR in the presence of 100 µM NADH was detected with increased concentration of Pdo All proteins (oxidized and reduced) were detected by staining with Coomassie brilliant blue as a loading control (upper panel) and mBBr-labeled proteins were detected by fluorescence illumination (lower panel) on 15% SDS-PAGE gels. M Molecular mass marker

Fig.S5Comparison of nucleotide sequences of mbh1 promotor regionsbetween T. onnurineusNA1 (TO_mbh1) and P. furiosus (PF_mbh1).The sequences of TO_mbh1 (GenBank accession no. CP000855) and PF_mbh1 (AE009950) were obtained from NCBI ( sequence alignment was conducted using the LALIGN program onweb server (

1