Appendix
Data of the IR spectra and elemental analysis of all new compounds.
1. Table of the combustion analysis data for the new compounds
Compound / Formula / C / H / NCalcd. / Found / Calcd. / Found / Calcd. / Found / Calcd. / Found
4 / C15H13N3O∙H2O / 69.00 / 69.33 / 5.57 / 5.34 / 15.61 / 15.64
7 / C25H31N5O / 71.91 / 72.13 / 7.48 / 7.41 / 16.77 / 16.45
5 / C25H31N5O / 71.91 / 71.96 / 7.48 / 7.49 / 16.77 / 16.53
8 / C15H13N3O / 71.70 / 72.06 / 5.21 / 5.13 / 16.72 / 16.42
6h / C22H28N3ClO3S / 58.71 / 58.87 / 6.27 / 6.39 / 9.34 / 9.44 / 7.88(Cl) / 7.79
6a / C23H31N3O3S / 64.40 / 64.34 / 7.27 / 7.34 / 9.78 / 9.70
6e / C23H31N3O4S / 62.00 / 61.96 / 7.01 / 7.04 / 9.43 / 9.28
6k / C24H32N4O4S / 60.99 / 60.86 / 6.83 / 6.76 / 11.86 / 11.83
6f / C24H33N3O4S / 62.72 / 62.67 / 7.24 / 7.49 / 9.14 / 9.22
11 / C14H15NO4S / 57.34 / 57.22 / 5.12 / 5.16 / 4.78 / 4.65
6f sulfate / C24H33N3O4S∙H2SO4∙3H2O / 47.06 / 47.00 / 6.70 / 6.98 / 6.68 / 6.87 / 10.48(S) / 10.65
6b / C24H33N3O3S / 64.99 / 65.01 / 7.50 / 7.20 / 9.42 / 9.41
10 / C14H15NO3S / 60.63 / 60.58 / 5.45 / 5.32 / 5.05 / 5.01
6i / C23H30N3O3SCl / 59.53 / 59.50 / 6.52 / 6.63 / 9.06 / 8.99 / 17.64(Cl) / 17.57
12 / C13H12NO3SCl / 52.44 / 52.42 / 4.06 / 4.07 / 4.70 / 4.65 / 11.91(Cl) / 11.92
6m / C25H34N4O4S∙H2O / 59.50 / 59.22 / 7.10 / 6.99 / 11.10 / 11.10
13 / C15H16N2O4S / 56.23 / 56.13 / 5.03 / 5.02 / 8.75 / 8.72
6c / C24H33N3O3S / 64.99 / 64.99 / 7.50 / 7.70 / 9.42 / 9.54
14 / C14H15NO3S / 60.63 / 60.38 / 5.45 / 5.42 / 5.05 / 4.91
6g / C24H33N3O4S / 62.32 / 62.32 / 7.24 / 7.33 / 9.14 / 9.05
15 / C14H15NO4S / 57.34 / 57.32 / 5.12 / 5.10 / 4.78 / 4.65
6j / C23H30N3O3SCl / 59.53 / 59.37 / 6.52 / 6.54 / 9.06 / 9.00 / 7.64(Cl) / 7.59
16 / C13H12NO3SCl / 52.44 / 52.53 / 4.06 / 4.00 / 4.70 / 4.78 / 11.91(Cl) / 11.88
6n / C25H34N4O4S ∙0.5H2O / 60.58 / 60.58 / 7.12 / 7.18 / 11.30 / 11.42
17 / C15H16N2O4S / 56.23 / 56.21 / 5.03 / 4.99 / 8.75 / 8.74
6d / C25H35N3O3S / 65.61 / 65.46 / 7.70 / 7.80 / 9.18 / 8.95
6p / C28H35N3O3S / 68.12 / 67.96 / 7.15 / 7.16 / 8.51 / 8.56
6o / C26H31N3O3S / 67.06 / 67.10 / 6.71 / 6.69 / 9.03 / 8.99
2. Table of the IR data of the new compounds
Compound / IR（ KBr, cm-1)4 / 3340, 3140, 3020, 1600, 1550,1500, 1460, 1405, 1350, 1250, 1200, 1170, 1125, 1100, 1010, 910, 835, 770
7 / 3430, 3200, 3060, 2970, 2780, 1620, 1580, 1535, 1500, 1475, 1460, 1360, 1330, 1160, 1140, 1125, 930, 890, 780
5 / 3430, 3070, 3030, 2970, 2880, 2790, 1615, 1570, 1545, 1500, 1480, 1400, 1360, 1265, 1125, 1040, 890, 775
8 / 3430, 2970, 2920, 2780, 1610, 1545, 1435, 1360, 1290, 1230, 1100, 925, 840, 770
6h / 3440, 2970, 2880, 2820, 2600, 1610, 1590, 1460, 1415, 1330, 1300, 1280, 1240, 1160, 1100, 925, 845, 750
6a / 3400, 2960, 2880, 2800, 1625, 1500, 1420, 1390, 1345, 1330, 1255, 1120, 1005, 940, 905, 880, 845, 810
6e / 2980, 2880, 2800, 2660, 1600, 1585,1500, 1465, 1410, 1330, 1265, 1160, 1100, 1035, 1015, 925, 840, 810
6k / 3350, 3260, 2960, 2880, 2790, 1690, 1600, 1535, 1475, 1400, 1320, 1260, 1170, 1100, 1020, 900, 835, 725
6f / 3158, 2963, 2808, 1596, 1494, 1329, 1297, 1251, 1159, 1097, 802, 561
11 / 3241, 2920, 2850, 1594, 1500, 1460, 1350, 1310, 1250, 1160, 1155, 1060, 1050, 1000, 850, 837, 719, 563
6f sulfate / 3430, 2969, 1648, 1595, 1496, 1456, 1326, 1302, 1257, 1155, 1121, 1063, 1025, 843, 619, 558
6b / 3400, 2965, 2880, 2800, 1600, 1465, 1370, 1290, 1180, 1160, 1130, 1035, 1000, 890, 850, 825
10 / 3410, 2965, 2880, 1465, 1370, 1290, 1180, 1165, 1130, 1035, 950, 890, 825,
6i / 3500, 2960, 2880, 2800, 2740, 1610, 1585, 1570, 1420, 1415, 1390, 1310, 1235, 1200, 1150, 1100, 1050, 945, 840
12 / 3505, 2955, 2880, 2800, 2740, 1610, 1585, 1570, 1420, 1415, 1315, 1230, 1200, 1150, 1045, 945, 845
6m / 3500, 3250, 3180, 3100, 2960, 2820, 1635, 1590, 1530, 1470, 1400, 1320, 1270, 1155, 1090, 1040, 1000, 880, 840
13 / 3500, 3255, 3175, 3100, 2955, 2800, 1635, 1580, 1535, 1465, 1400, 1320, 1260, 1150, 1085, 1040, 880, 790
6c / 3400, 2960, 2880, 2770, 1595, 1465, 1405, 1330, 1280, 1225, 1160, 1120, 1085, 990, 960, 900, 830, 810
14 / 3400, 2950, 2880, 2770, 1595, 1465, 1400, 1320, 1270, 1225, 1165, 1120, 1080, 995, 905, 830, 810
6g / 3440, 2960, 2870, 2780, 1610, 1580, 1470, 1400, 1360, 1280, 1230, 1200, 1170, 1120, 1090, 1010, 995, 960, 940, 885, 820, 760
15 / 3300, 3160, 3020, 2960, 2870, 2820, 1680, 1590, 1540, 1460, 1400, 1370, 1340, 1230, 1150, 1110, 960, 825
6j / 3400, 2950, 2830, 2770, 1595, 1495, 1460, 1410, 1330, 1300, 1225, 1155, 1090, 990, 960, 900, 820
16 / 3400, 2950, 2830, 2770, 1495, 1460, 1410, 1330, 1300, 1225, 1155, 1095, 995, 950, 820
6n / 3440, 3300, 3240, 3160, 3020, 2960, 2870, 2820, 1680, 1590, 1540, 1460, 1370, 1340, 1210, 1160, 1115, 960, 825
17 / 3430, 3300, 3240, 3020, 2960, 2865, 2820, 1680, 1590, 1540, 1460, 1400, 1370, 1340, 1210, 1160, 1115, 965, 820
6d / 3410, 2970, 2880, 2800, 1600, 1515, 1460, 1370, 1290, 1180, 1160, 1130, 1090, 1000, 890, 850, 825, 755
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